Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films

J. M. Boulton; Gimtong T. Teowee; W. M. Bommersbach; Donald R. Uhlmann

doi:10.1117/12.132023

Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films

J. M. Boulton, Gimtong T. Teowee, W. M. Bommersbach, Donald R. Uhlmann

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

7 Scopus citations

Abstract

Sol-gel routes were developed to Ba₂NaNb₅O₁₅, BaTiO₃, Ba_0.8Pb_0.2TiO₃, Ba_0.8Sr_0.2TiO₃, Bi₄Ti₃O₁₂, LiNbO₃, LiTaO₃, Pb₅Ge₃O₁₁, PbTiO₃, Pb_0.85La_0.15Ti_0.96O₃, PbZr_0.2Ti_0.8O₃, WO₃ and ZnO thin films. Second harmonic generation (SHG) from these films deposited on fused SiO₂ was investigated as a function of processing temperature. The SHG values were found to be related to the second-order nonlinear optical susceptibilities of the bulk materials, and dependent on the crystal size and crystalline orientation of the film. The highest SHG observed was from PbTiO₃ films which is consistent with the fact that the d-coefficient of PbTiO₃ is the highest among that of any room temperature ferroelectric. The poor SHG activity of BaTiO₃-based films was due to the very small grain size of the sol-gel derived material.

Original language	English (US)
Title of host publication	Proceedings of SPIE - The International Society for Optical Engineering
Publisher	Publ by Int Soc for Optical Engineering
Pages	292-303
Number of pages	12
ISBN (Print)	0819409316, 9780819409317
DOIs	https://doi.org/10.1117/12.132023
State	Published - 1992
Event	Sol-Gel Optics II - San Diego, CA, USA Duration: Jul 20 1992 → Jul 22 1992

Publication series

Name	Proceedings of SPIE - The International Society for Optical Engineering
Volume	1758
ISSN (Print)	0277-786X

Other

Other	Sol-Gel Optics II
City	San Diego, CA, USA
Period	7/20/92 → 7/22/92

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Computer Science Applications
Applied Mathematics
Electrical and Electronic Engineering

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10.1117/12.132023

Cite this

Boulton, J. M., Teowee, G. T., Bommersbach, W. M., & Uhlmann, D. R. (1992). Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films. In Proceedings of SPIE - The International Society for Optical Engineering (pp. 292-303). (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 1758). Publ by Int Soc for Optical Engineering. https://doi.org/10.1117/12.132023

Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films. / Boulton, J. M.; Teowee, Gimtong T.; Bommersbach, W. M. et al.
Proceedings of SPIE - The International Society for Optical Engineering. Publ by Int Soc for Optical Engineering, 1992. p. 292-303 (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 1758).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Boulton, JM, Teowee, GT, Bommersbach, WM & Uhlmann, DR 1992, Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films. in Proceedings of SPIE - The International Society for Optical Engineering. Proceedings of SPIE - The International Society for Optical Engineering, vol. 1758, Publ by Int Soc for Optical Engineering, pp. 292-303, Sol-Gel Optics II, San Diego, CA, USA, 7/20/92. https://doi.org/10.1117/12.132023

Boulton JM, Teowee GT, Bommersbach WM, Uhlmann DR. Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films. In Proceedings of SPIE - The International Society for Optical Engineering. Publ by Int Soc for Optical Engineering. 1992. p. 292-303. (Proceedings of SPIE - The International Society for Optical Engineering). doi: 10.1117/12.132023

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title = "Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films",

abstract = "Sol-gel routes were developed to Ba2NaNb5O15, BaTiO3, Ba0.8Pb 0.2TiO3, Ba0.8Sr0.2TiO3, Bi4Ti3O12, LiNbO3, LiTaO 3, Pb5Ge3O11, PbTiO3, Pb0.85La0.15Ti0.96O3, PbZr 0.2Ti0.8O3, WO3 and ZnO thin films. Second harmonic generation (SHG) from these films deposited on fused SiO2 was investigated as a function of processing temperature. The SHG values were found to be related to the second-order nonlinear optical susceptibilities of the bulk materials, and dependent on the crystal size and crystalline orientation of the film. The highest SHG observed was from PbTiO3 films which is consistent with the fact that the d-coefficient of PbTiO3 is the highest among that of any room temperature ferroelectric. The poor SHG activity of BaTiO3-based films was due to the very small grain size of the sol-gel derived material.",

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N2 - Sol-gel routes were developed to Ba2NaNb5O15, BaTiO3, Ba0.8Pb 0.2TiO3, Ba0.8Sr0.2TiO3, Bi4Ti3O12, LiNbO3, LiTaO 3, Pb5Ge3O11, PbTiO3, Pb0.85La0.15Ti0.96O3, PbZr 0.2Ti0.8O3, WO3 and ZnO thin films. Second harmonic generation (SHG) from these films deposited on fused SiO2 was investigated as a function of processing temperature. The SHG values were found to be related to the second-order nonlinear optical susceptibilities of the bulk materials, and dependent on the crystal size and crystalline orientation of the film. The highest SHG observed was from PbTiO3 films which is consistent with the fact that the d-coefficient of PbTiO3 is the highest among that of any room temperature ferroelectric. The poor SHG activity of BaTiO3-based films was due to the very small grain size of the sol-gel derived material.

AB - Sol-gel routes were developed to Ba2NaNb5O15, BaTiO3, Ba0.8Pb 0.2TiO3, Ba0.8Sr0.2TiO3, Bi4Ti3O12, LiNbO3, LiTaO 3, Pb5Ge3O11, PbTiO3, Pb0.85La0.15Ti0.96O3, PbZr 0.2Ti0.8O3, WO3 and ZnO thin films. Second harmonic generation (SHG) from these films deposited on fused SiO2 was investigated as a function of processing temperature. The SHG values were found to be related to the second-order nonlinear optical susceptibilities of the bulk materials, and dependent on the crystal size and crystalline orientation of the film. The highest SHG observed was from PbTiO3 films which is consistent with the fact that the d-coefficient of PbTiO3 is the highest among that of any room temperature ferroelectric. The poor SHG activity of BaTiO3-based films was due to the very small grain size of the sol-gel derived material.

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Second-harmonic generation from sol-gel-derived ferroelectric and piezoelectric thin films

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