TY - JOUR
T1 - Radiocarbon bomb-peak signal in tree-rings from the tropical Andes register low latitude atmospheric dynamics in the Southern Hemisphere
AU - Ancapichún, Santiago
AU - De Pol-Holz, Ricardo
AU - Christie, Duncan A.
AU - Santos, Guaciara M.
AU - Collado-Fabbri, Silvana
AU - Garreaud, René
AU - Lambert, Fabrice
AU - Orfanoz-Cheuquelaf, Andrea
AU - Rojas, Maisa
AU - Southon, John
AU - Turnbull, Jocelyn C.
AU - Creasman, Pearce Paul
N1 - Funding Information:
We would like to thank all the personnel at the Keck Radiocarbon Facility of the University of California, Irvine for their continuous õsupport and laboratory help. Funding for this study came from the Chilean Agencia Nacional de Investigación y Desarrollo (ANID) Fondecyt grants # 1140536 , # 1201810 and 1201411 ; ANID FONDAP 15110009 (CR) 2 and ICM NC120066 . SA was partially supported by the ANID doctoral scholarship 21140194 .
Funding Information:
We would like to thank all the personnel at the Keck Radiocarbon Facility of the University of California, Irvine for their continuous ?support and laboratory help. Funding for this study came from the Chilean Agencia Nacional de Investigaci?n y Desarrollo (ANID) Fondecyt grants #1140536, #1201810 and 1201411; ANID FONDAP 15110009 (CR)2 and ICM NC120066. SA was partially supported by the ANID doctoral scholarship 21140194.
Publisher Copyright:
© 2021 Elsevier B.V.
PY - 2021/6/20
Y1 - 2021/6/20
N2 - South American tropical climate is strongly related to the tropical low-pressure belt associated with the South American monsoon system. Despite its central societal role as a modulating agent of rainfall in tropical South America, its long-term dynamical variability is still poorly understood. Here we combine a new (and world's highest) tree-ring 14C record from the Altiplano plateau in the central Andes with other 14C records from the Southern Hemisphere during the second half of the 20th century in order to elucidate the latitudinal gradients associated with the dissemination of the bomb 14C signal. Our tree-ring 14C record faithfully captured the bomb signal of the 1960's with an excellent match to atmospheric 14C measured in New Zealand but with significant differences with a recent record from Southeast Brazil located at almost equal latitude. These results imply that the spreading of the bomb signal throughout the Southern Hemisphere was a complex process that depended on atmospheric dynamics and surface topography generating reversals on the expected north-south gradient in certain years. We applied air-parcel modeling based on climate data to disentangle their different geographical provenances and their preformed (reservoir affected) radiocarbon content. We found that air parcel trajectories arriving at the Altiplano during the bomb period were sourced i) from the boundary layer in contact with the Pacific Ocean (41%), ii) from the upper troposphere (air above the boundary layer, with no contact with oceanic or continental carbon reservoirs) (38%) and iii) from the Amazon basin (21%). Based on these results we estimated the ∆14C endmember values for the different carbon reservoirs affecting our record which suggest that the Amazon basin biospheric 14C isoflux could have been reversed from negative to positive as early as the beginning of the 1970's. This would imply a much faster carbon turnover rate in the Amazon than previously modelled.
AB - South American tropical climate is strongly related to the tropical low-pressure belt associated with the South American monsoon system. Despite its central societal role as a modulating agent of rainfall in tropical South America, its long-term dynamical variability is still poorly understood. Here we combine a new (and world's highest) tree-ring 14C record from the Altiplano plateau in the central Andes with other 14C records from the Southern Hemisphere during the second half of the 20th century in order to elucidate the latitudinal gradients associated with the dissemination of the bomb 14C signal. Our tree-ring 14C record faithfully captured the bomb signal of the 1960's with an excellent match to atmospheric 14C measured in New Zealand but with significant differences with a recent record from Southeast Brazil located at almost equal latitude. These results imply that the spreading of the bomb signal throughout the Southern Hemisphere was a complex process that depended on atmospheric dynamics and surface topography generating reversals on the expected north-south gradient in certain years. We applied air-parcel modeling based on climate data to disentangle their different geographical provenances and their preformed (reservoir affected) radiocarbon content. We found that air parcel trajectories arriving at the Altiplano during the bomb period were sourced i) from the boundary layer in contact with the Pacific Ocean (41%), ii) from the upper troposphere (air above the boundary layer, with no contact with oceanic or continental carbon reservoirs) (38%) and iii) from the Amazon basin (21%). Based on these results we estimated the ∆14C endmember values for the different carbon reservoirs affecting our record which suggest that the Amazon basin biospheric 14C isoflux could have been reversed from negative to positive as early as the beginning of the 1970's. This would imply a much faster carbon turnover rate in the Amazon than previously modelled.
KW - Atmospheric circulation
KW - Carbon reservoir effect
KW - Radiocarbon
KW - Southern hemisphere
KW - Tree-rings
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UR - http://www.scopus.com/inward/citedby.url?scp=85101128522&partnerID=8YFLogxK
U2 - 10.1016/j.scitotenv.2021.145126
DO - 10.1016/j.scitotenv.2021.145126
M3 - Article
C2 - 33611001
AN - SCOPUS:85101128522
SN - 0048-9697
VL - 774
JO - Science of the Total Environment
JF - Science of the Total Environment
M1 - 145126
ER -