Quasi-phase-matched third harmonic generation in organic multilayers

Jiung Kim, Ch S.S.Pavan Kumar, Myoungsik Cha, Heejoo Choi, Kyung Jo Kim, N. Peyghambarian

Research output: Contribution to journalArticlepeer-review

4 Scopus citations


We report the first realization of quasi-phase-matched (QPM) third harmonic generation in isotropic polymer films. Spin-coated thin films of ethyl-violet molecules dispersed in a polymer host (EV) were used as cubic nonlinear optical media because of their transparency at both the fundamental (1230 nm) and the third harmonic (410 nm) wavelengths. A passive layer of a UV-curable material was formed to compensate the phase shift between the two light waves after propagating through each EV layer. We fabricated a series of samples with 1~4 EV layers (0~3 alternatingly coated passive layers). The third harmonic output power showed a quadratic increase with the number of layers, providing a strong evidence for successful quasi-phase-matching. A conversion efficiency of 0.15% was observed with a 190 fs pulse input.

Original languageEnglish (US)
Article number16419
JournalScientific reports
Issue number1
StatePublished - Dec 1 2018

ASJC Scopus subject areas

  • General


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