Abstract
We present experimental results and a theoretical framework for understanding the ionization dynamics in atoms exposed to XUV attosecond pulse trains and strong multi-cycle infrared (IR) fields. We invoke the Floquet formalism to model dressed atomic states as a manifold of Fourier components spaced by the laser frequency. In XUV-IR pump-probe measurements, we observe that the ionization yield oscillates due to quantum interference between photo-excitation paths to a Floquet state. We show that the intensity-dependent shifts of atomic structure modify the ionization channels and the associated interference phase. We extract this phase variation and compare it with simulations. These results provide a comprehensive description of the two-color ionization process and enable new schemes for control of attosecond ionization and fragmentation dynamics.
Original language | English (US) |
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Pages (from-to) | 139-148 |
Number of pages | 10 |
Journal | Chemical Physics |
Volume | 414 |
DOIs | |
State | Published - Mar 12 2013 |
Keywords
- Attosecond
- Floquet
- Photoionization
- Strong fields
ASJC Scopus subject areas
- General Physics and Astronomy
- Physical and Theoretical Chemistry