TY - JOUR
T1 - Impacts of regional wind circulations on aerosol pollution and planetary boundary layer structure in Metro Manila, Philippines
AU - Cruz, Melliza Templonuevo
AU - Simpas, James Bernard
AU - Sorooshian, Armin
AU - Betito, Grace
AU - Cambaliza, Maria Obiminda L.
AU - Collado, Jarl Tynan
AU - Eloranta, Edwin W.
AU - Holz, Robert
AU - Topacio, Xzann Garry Vincent
AU - Del Socorro, Jundy
AU - Bagtasa, Gerry
N1 - Publisher Copyright:
© 2022 Elsevier Ltd
PY - 2023/1/15
Y1 - 2023/1/15
N2 - Fine particulate matter (PM2.5) concentrations in Metro Manila, Philippines have consistently exceeded the guideline values set by the World Health Organization (WHO). Although there has been much progress in understanding the components and sources of PM2.5, limited research has been done on the influence of meteorological factors. In particular, the influence of the planetary boundary layer height (PBLH) on PM2.5 concentration has not been studied due to inadequate observations. From January 2019–June 2020, measurements from a High Spectral Resolution Lidar (HSRL) filled this gap and allowed for PBLH estimation and aerosol typing. This paper investigates the roles of PBLH and regional and local wind circulations on the temporal evolution of aerosol pollution. Results show that daytime and nighttime PBLH variability is associated with solar heating and radiative cooling, respectively. Cloud-free conditions during the dry season yield a higher PBL growth rate than during the wet season when lower daytime and elevated nighttime PBLH are observed. Lower PM2.5 levels are generally observed during daytime when PBLH is at its maximum. However, the PBLH has a significant inverse correlation with PM2.5 only in the months of December-January-February. We find that horizontal directional wind shear between synoptic and mesoscale circulations confounds the PM2.5 - PBLH relationship by creating stagnant conditions conducive to aerosol accumulation. The lower 20% of PM2.5 concentrations occur during the prevalence of strong monsoon winds. On the other hand, the upper 80% are found during the occurrence of compound mesoscale winds (i.e., sea/land/lake/valley/mountain breezes and channeling monsoon winds). In addition, mountain breeze is found to be associated with lifting of aerosols, resulting in multi-layering within the PBL. The findings in the present study emphasize the role of complex topography and mesoscale scale winds arising from the landscape on aerosol pollution variability.
AB - Fine particulate matter (PM2.5) concentrations in Metro Manila, Philippines have consistently exceeded the guideline values set by the World Health Organization (WHO). Although there has been much progress in understanding the components and sources of PM2.5, limited research has been done on the influence of meteorological factors. In particular, the influence of the planetary boundary layer height (PBLH) on PM2.5 concentration has not been studied due to inadequate observations. From January 2019–June 2020, measurements from a High Spectral Resolution Lidar (HSRL) filled this gap and allowed for PBLH estimation and aerosol typing. This paper investigates the roles of PBLH and regional and local wind circulations on the temporal evolution of aerosol pollution. Results show that daytime and nighttime PBLH variability is associated with solar heating and radiative cooling, respectively. Cloud-free conditions during the dry season yield a higher PBL growth rate than during the wet season when lower daytime and elevated nighttime PBLH are observed. Lower PM2.5 levels are generally observed during daytime when PBLH is at its maximum. However, the PBLH has a significant inverse correlation with PM2.5 only in the months of December-January-February. We find that horizontal directional wind shear between synoptic and mesoscale circulations confounds the PM2.5 - PBLH relationship by creating stagnant conditions conducive to aerosol accumulation. The lower 20% of PM2.5 concentrations occur during the prevalence of strong monsoon winds. On the other hand, the upper 80% are found during the occurrence of compound mesoscale winds (i.e., sea/land/lake/valley/mountain breezes and channeling monsoon winds). In addition, mountain breeze is found to be associated with lifting of aerosols, resulting in multi-layering within the PBL. The findings in the present study emphasize the role of complex topography and mesoscale scale winds arising from the landscape on aerosol pollution variability.
KW - Aerosols
KW - Boundary layer
KW - Horizontal wind shear
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U2 - 10.1016/j.atmosenv.2022.119455
DO - 10.1016/j.atmosenv.2022.119455
M3 - Article
AN - SCOPUS:85143496704
SN - 1352-2310
VL - 293
JO - Atmospheric Environment
JF - Atmospheric Environment
M1 - 119455
ER -