Friction dependence on growth conditions in epitaxial films

Anne E. Murdaugh; Srinivas Manne

doi:10.1021/la9008448

Friction dependence on growth conditions in epitaxial films

Anne E. Murdaugh, Srinivas Manne

Physics

Research output: Contribution to journal › Article › peer-review

2 Scopus citations

Abstract

In investigating the growth kinetics of epitaxial films in situ by force microscopy, we have observed several instances where the lateral force contrast on the growing monolayer exhibits a strong dependence on the driving force for growth (i.e., solute concentration). We present results for three epitaxial growth systems in aqueous solutions: CaSO₃ on CaCO₃, PbSO₄ on BaSO₄, and BaSO₃ on BaSO₄. In each system, material grown at higher solute concentrations exhibits a friction higher than that of material grown at lower concentrations. These observations suggest a link between defect density and friction contrast in growing epitaxial films. An additional time-dependent behavior is observed in the CaSO₃/CaCO₃ system, indicating an annealing process.

Original language	English (US)
Pages (from-to)	9792-9796
Number of pages	5
Journal	Langmuir
Volume	25
Issue number	17
DOIs	https://doi.org/10.1021/la9008448
State	Published - Sep 1 2009

ASJC Scopus subject areas

General Materials Science
Condensed Matter Physics
Surfaces and Interfaces
Spectroscopy
Electrochemistry

Access to Document

10.1021/la9008448

Cite this

@article{5837b231309c48a6978fb64c35c725c4,

title = "Friction dependence on growth conditions in epitaxial films",

abstract = "In investigating the growth kinetics of epitaxial films in situ by force microscopy, we have observed several instances where the lateral force contrast on the growing monolayer exhibits a strong dependence on the driving force for growth (i.e., solute concentration). We present results for three epitaxial growth systems in aqueous solutions: CaSO3 on CaCO3, PbSO4 on BaSO4, and BaSO3 on BaSO4. In each system, material grown at higher solute concentrations exhibits a friction higher than that of material grown at lower concentrations. These observations suggest a link between defect density and friction contrast in growing epitaxial films. An additional time-dependent behavior is observed in the CaSO3/CaCO3 system, indicating an annealing process.",

author = "Murdaugh, {Anne E.} and Srinivas Manne",

year = "2009",

month = sep,

day = "1",

doi = "10.1021/la9008448",

language = "English (US)",

volume = "25",

pages = "9792--9796",

journal = "Langmuir",

issn = "0743-7463",

publisher = "American Chemical Society",

number = "17",

}

TY - JOUR

T1 - Friction dependence on growth conditions in epitaxial films

AU - Murdaugh, Anne E.

AU - Manne, Srinivas

PY - 2009/9/1

Y1 - 2009/9/1

N2 - In investigating the growth kinetics of epitaxial films in situ by force microscopy, we have observed several instances where the lateral force contrast on the growing monolayer exhibits a strong dependence on the driving force for growth (i.e., solute concentration). We present results for three epitaxial growth systems in aqueous solutions: CaSO3 on CaCO3, PbSO4 on BaSO4, and BaSO3 on BaSO4. In each system, material grown at higher solute concentrations exhibits a friction higher than that of material grown at lower concentrations. These observations suggest a link between defect density and friction contrast in growing epitaxial films. An additional time-dependent behavior is observed in the CaSO3/CaCO3 system, indicating an annealing process.

AB - In investigating the growth kinetics of epitaxial films in situ by force microscopy, we have observed several instances where the lateral force contrast on the growing monolayer exhibits a strong dependence on the driving force for growth (i.e., solute concentration). We present results for three epitaxial growth systems in aqueous solutions: CaSO3 on CaCO3, PbSO4 on BaSO4, and BaSO3 on BaSO4. In each system, material grown at higher solute concentrations exhibits a friction higher than that of material grown at lower concentrations. These observations suggest a link between defect density and friction contrast in growing epitaxial films. An additional time-dependent behavior is observed in the CaSO3/CaCO3 system, indicating an annealing process.

UR - http://www.scopus.com/inward/record.url?scp=69949163637&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=69949163637&partnerID=8YFLogxK

U2 - 10.1021/la9008448

DO - 10.1021/la9008448

M3 - Article

C2 - 19663430

AN - SCOPUS:69949163637

SN - 0743-7463

VL - 25

SP - 9792

EP - 9796

JO - Langmuir

JF - Langmuir

IS - 17

ER -

Friction dependence on growth conditions in epitaxial films

Abstract

ASJC Scopus subject areas

Access to Document

Other files and links

Fingerprint

Cite this