Abstract
Short laser pulses are able to generate material excitations with a well-defined phase which is imposed by the optical excitation source. The generated coherent superposition state be described as an optical polarization which exists only in non-equilibrium situations. The coherence, i.e., the phase relations between the optical transitions that originate from the excitation, leads to several interesting effects in time-resolved linear and nonlinear optical spectroscopy. In this article, the basic principles that underlie these coherent transients are introduced and several examples are presented.
Original language | English (US) |
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Title of host publication | Encyclopedia of Modern Optics |
Publisher | Elsevier |
Pages | 264-277 |
Number of pages | 14 |
Volume | 1-5 |
ISBN (Electronic) | 9780128149829 |
ISBN (Print) | 9780128092835 |
DOIs | |
State | Published - Jan 1 2018 |
Externally published | Yes |
Keywords
- Bloch equations
- Coherent control
- Coherent photocurrents
- Dephasing
- Free-induction decay
- Interference
- Light-matter interaction
- Multidimensional fourier transform spectroscopy
- Nonlinear optical spectroscopy
- Optical polarization
- Photon echo
- Quantum beats
- Radiative decay
- Semiconductor bloch equations
- Spectral oscillations
- Superradiance
ASJC Scopus subject areas
- General Engineering
- General Materials Science