Abstract
We present analytical results and kinetic Monte Carlo simulations for the mobility and microscopic structure of solid-on-solid (SOS) interfaces driven far from equilibrium by an external force, such as an applied field or (electro)chemical potential difference. The interfaces evolve under a specific stochastic dynamics with a local energy barrier (an Arrhenius dynamics), known as the transition dynamics approximation (TDA). We calculate the average height of steps on the interface, the average interface velocity, and the skewness of the interface as functions of the driving force and the height of the energy barrier. We find that the microscopic interface structure depends quite strongly on the barrier height. As the barrier becomes higher, the local interface width decreases and the skewness increases, suggesting increasing short-range correlations between the step heights.
Original language | English (US) |
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Pages (from-to) | 207-210 |
Number of pages | 4 |
Journal | Journal of Molecular Structure: THEOCHEM |
Volume | 769 |
Issue number | 1-3 |
DOIs | |
State | Published - Sep 14 2006 |
Keywords
- Arrhenius dynamics
- Interface structure
- Monte Carlo simulation
ASJC Scopus subject areas
- Biochemistry
- Condensed Matter Physics
- Physical and Theoretical Chemistry