Extended squaraine dyes with large two-photon absorption cross-sections

Sung Jae Chung; Shijun Zheng; Toru Odani; Luca Beverina; Jie Fu; Lazaro A. Padilha; Arianna Biesso; Joel M. Hales; Xiaowei Zhan; Karin Schmidt; Aijun Ye; Egbert Zojer; Stephen Barlow; David J. Hagan; Eric W. Van Stryland; Yuanping Yi; Zhigang Shuai; Giorgio A. Pagani; Jean Luc Brédas; Joseph W. Perry; Seth R. Marder

doi:10.1021/ja065556m

Extended squaraine dyes with large two-photon absorption cross-sections

Sung Jae Chung
, Shijun Zheng
, Toru Odani
, Luca Beverina
, Jie Fu
, Lazaro A. Padilha
, Arianna Biesso
, Joel M. Hales
, Xiaowei Zhan
, Karin Schmidt
, Aijun Ye
, Egbert Zojer
, Stephen Barlow
, David J. Hagan
, Eric W. Van Stryland
, Yuanping Yi
, Zhigang Shuai
, Giorgio A. Pagani
, Jean Luc Brédas
, Joseph W. Perry

Seth R. Marder

Research output: Contribution to journal › Article › peer-review

227 Scopus citations

Abstract

Extended bis(donor)-substituted squaraine chromophores exhibit very high two-photon cross-sections (as high as 33000 GM) in the near-IR; these can be attributed to the combination of large transition dipoles with small detuning energies. The modulus of the third-order nonlinear optical susceptibility at 1.3 μm has been found to be 7.0 × 10^-11 esu for one of these chromophores.

Original language	English (US)
Pages (from-to)	14444-14445
Number of pages	2
Journal	Journal of the American Chemical Society
Volume	128
Issue number	45
DOIs	https://doi.org/10.1021/ja065556m
State	Published - Nov 15 2006
Externally published	Yes

ASJC Scopus subject areas

Catalysis
General Chemistry
Biochemistry
Colloid and Surface Chemistry

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10.1021/ja065556m

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Chung, S. J., Zheng, S., Odani, T., Beverina, L., Fu, J., Padilha, L. A., Biesso, A., Hales, J. M., Zhan, X., Schmidt, K., Ye, A., Zojer, E., Barlow, S., Hagan, D. J., Van Stryland, E. W., Yi, Y., Shuai, Z., Pagani, G. A., Brédas, J. L., ... Marder, S. R. (2006). Extended squaraine dyes with large two-photon absorption cross-sections. Journal of the American Chemical Society, 128(45), 14444-14445. https://doi.org/10.1021/ja065556m

Chung, SJ, Zheng, S, Odani, T, Beverina, L, Fu, J, Padilha, LA, Biesso, A, Hales, JM, Zhan, X, Schmidt, K, Ye, A, Zojer, E, Barlow, S, Hagan, DJ, Van Stryland, EW, Yi, Y, Shuai, Z, Pagani, GA, Brédas, JL, Perry, JW & Marder, SR 2006, 'Extended squaraine dyes with large two-photon absorption cross-sections', Journal of the American Chemical Society, vol. 128, no. 45, pp. 14444-14445. https://doi.org/10.1021/ja065556m

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title = "Extended squaraine dyes with large two-photon absorption cross-sections",

abstract = "Extended bis(donor)-substituted squaraine chromophores exhibit very high two-photon cross-sections (as high as 33000 GM) in the near-IR; these can be attributed to the combination of large transition dipoles with small detuning energies. The modulus of the third-order nonlinear optical susceptibility at 1.3 μm has been found to be 7.0 × 10-11 esu for one of these chromophores.",

author = "Chung, \{Sung Jae\} and Shijun Zheng and Toru Odani and Luca Beverina and Jie Fu and Padilha, \{Lazaro A.\} and Arianna Biesso and Hales, \{Joel M.\} and Xiaowei Zhan and Karin Schmidt and Aijun Ye and Egbert Zojer and Stephen Barlow and Hagan, \{David J.\} and \{Van Stryland\}, \{Eric W.\} and Yuanping Yi and Zhigang Shuai and Pagani, \{Giorgio A.\} and Br{\'e}das, \{Jean Luc\} and Perry, \{Joseph W.\} and Marder, \{Seth R.\}",

year = "2006",

month = nov,

day = "15",

doi = "10.1021/ja065556m",

language = "English (US)",

volume = "128",

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journal = "Journal of the American Chemical Society",

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T1 - Extended squaraine dyes with large two-photon absorption cross-sections

AU - Chung, Sung Jae

AU - Zheng, Shijun

AU - Odani, Toru

AU - Beverina, Luca

AU - Fu, Jie

AU - Padilha, Lazaro A.

AU - Biesso, Arianna

AU - Hales, Joel M.

AU - Zhan, Xiaowei

AU - Schmidt, Karin

AU - Ye, Aijun

AU - Zojer, Egbert

AU - Barlow, Stephen

AU - Hagan, David J.

AU - Van Stryland, Eric W.

AU - Yi, Yuanping

AU - Shuai, Zhigang

AU - Pagani, Giorgio A.

AU - Brédas, Jean Luc

AU - Perry, Joseph W.

AU - Marder, Seth R.

PY - 2006/11/15

Y1 - 2006/11/15

N2 - Extended bis(donor)-substituted squaraine chromophores exhibit very high two-photon cross-sections (as high as 33000 GM) in the near-IR; these can be attributed to the combination of large transition dipoles with small detuning energies. The modulus of the third-order nonlinear optical susceptibility at 1.3 μm has been found to be 7.0 × 10-11 esu for one of these chromophores.

AB - Extended bis(donor)-substituted squaraine chromophores exhibit very high two-photon cross-sections (as high as 33000 GM) in the near-IR; these can be attributed to the combination of large transition dipoles with small detuning energies. The modulus of the third-order nonlinear optical susceptibility at 1.3 μm has been found to be 7.0 × 10-11 esu for one of these chromophores.

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U2 - 10.1021/ja065556m

DO - 10.1021/ja065556m

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SN - 0002-7863

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EP - 14445

JO - Journal of the American Chemical Society

JF - Journal of the American Chemical Society

IS - 45

ER -

Extended squaraine dyes with large two-photon absorption cross-sections

Abstract

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